TARFOX_UWC131A_SUNP Data Set was collected from the 6-channel Sun Photometer flown on the University of Washington C-131A aircraft during the Tropospheric Aerosol Radiative Forcing Observational eXperiment (TARFOX) mission. The TARFOX Intensive Field Campaign was conducted July 10-31, 1996. It included coordinated measurements from four satellites (GOES-8, NOAA-14, ERS-2, LANDSAT), four aircraft (ER-2, C-130, C-131A, and a modified Cessna), land sites, and ships. A variety of aerosol conditions was sampled, ranging from relatively clean behind frontal passages to moderately polluted with aerosol optical depths exceeding 0.5 at mid-visible wavelengths. Gradients of aerosol optical thickness were sampled to aid in isolating aerosol effects from other radiative effects and to more tightly constrain closure tests, including those of satellite retrievals. Early results from TARFOX include demonstration of the unexpected importance of carbonaceous compounds and water condensed on aerosol in the US mid-Atlantic haze plume, chemical apportionment of the aerosol optical depth, measurements of the downward component of aerosol radiative forcing, and agreement between forcing measurements and calculations.